Multi-modal impedance and X-ray characterization enables simultaneous detection of bulk and interfacial crystallization

Nikolaus Doppelhammer; Daniel Spira; Anjul Rais; Dries Vandenabeele; Wauter Wangermez; Charles McMonagle; Dmitry Chernyshov; Eric Breynaert

doi:10.1039/d5cc03808a

Multi-modal impedance and X-ray characterization enables simultaneous detection of bulk and interfacial crystallization

Nikolaus Doppelhammer^*
, Daniel Spira
, Anjul Rais
, Dries Vandenabeele
, Wauter Wangermez
, Charles McMonagle
, Dmitry Chernyshov
, Eric Breynaert

^*Corresponding author for this work

Institute of Microelectronics and Microsensors

Research output: Contribution to journal › Article › peer-review

Abstract

A multi-modal platform enabling simultaneous impedance spectroscopy and X-ray scattering is presented. When applied to zeolite crystallization, four-electrode impedance measurements reliably track bulk crystallization kinetics in agreement with X-ray diffraction, while two-electrode impedance data reveal artefacts from electrode passivation.

Original language	English
Pages (from-to)	14919-14922
Number of pages	4
Journal	Chemical Communications
Issue number	77
DOIs	https://doi.org/10.1039/d5cc03808a
Publication status	Published - 19 Aug 2025

Fields of science

202028 Microelectronics
202027 Mechatronics
202 Electrical Engineering, Electronics, Information Engineering
202037 Signal processing
202036 Sensor systems
104003 Inorganic chemistry
104005 Electrochemistry
104011 Materials chemistry
104024 X-ray structural analysis

JKU Focus areas

Digital Transformation

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10.1039/d5cc03808a

https://doi.org/10.1039/D5CC03808ALicence: CC BY-NC

Cite this

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title = "Multi-modal impedance and X-ray characterization enables simultaneous detection of bulk and interfacial crystallization",

abstract = "A multi-modal platform enabling simultaneous impedance spectroscopy and X-ray scattering is presented. When applied to zeolite crystallization, four-electrode impedance measurements reliably track bulk crystallization kinetics in agreement with X-ray diffraction, while two-electrode impedance data reveal artefacts from electrode passivation.",

author = "Nikolaus Doppelhammer and Daniel Spira and Anjul Rais and Dries Vandenabeele and Wauter Wangermez and Charles McMonagle and Dmitry Chernyshov and Eric Breynaert",

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doi = "10.1039/d5cc03808a",

language = "English",

pages = "14919--14922",

journal = "Chemical Communications",

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AU - Doppelhammer, Nikolaus

AU - Spira, Daniel

AU - Rais, Anjul

AU - Vandenabeele, Dries

AU - Wangermez, Wauter

AU - McMonagle, Charles

AU - Chernyshov, Dmitry

AU - Breynaert, Eric

PY - 2025/8/19

Y1 - 2025/8/19

N2 - A multi-modal platform enabling simultaneous impedance spectroscopy and X-ray scattering is presented. When applied to zeolite crystallization, four-electrode impedance measurements reliably track bulk crystallization kinetics in agreement with X-ray diffraction, while two-electrode impedance data reveal artefacts from electrode passivation.

AB - A multi-modal platform enabling simultaneous impedance spectroscopy and X-ray scattering is presented. When applied to zeolite crystallization, four-electrode impedance measurements reliably track bulk crystallization kinetics in agreement with X-ray diffraction, while two-electrode impedance data reveal artefacts from electrode passivation.

UR - https://www.scopus.com/pages/publications/105016805480

U2 - 10.1039/d5cc03808a

DO - 10.1039/d5cc03808a

M3 - Article

SN - 1359-7345

SP - 14919

EP - 14922

JO - Chemical Communications

JF - Chemical Communications

IS - 77

ER -

Multi-modal impedance and X-ray characterization enables simultaneous detection of bulk and interfacial crystallization

Abstract

Fields of science

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Other files and links

MEmeZe - Bewegte Elektroden treffen auf Zeolithe

ESRF BM01 - Investigating Early Zeolite Nucleation Stages in Hydrated Silicate Ionic Liquids Using In Situ SAXS, WAXS, and Impedance Spectroscopy

ESRF BM26 - Assessing HSIL zeolite crystallization in mixed cation systems

Cite this

Multi-modal impedance and X-ray characterization enables simultaneous detection of bulk and interfacial crystallization

Abstract

Fields of science

JKU Focus areas

Access to Document

Other files and links

Projects

MEmeZe - Bewegte Elektroden treffen auf Zeolithe

ESRF BM01 - Investigating Early Zeolite Nucleation Stages in Hydrated Silicate Ionic Liquids Using In Situ SAXS, WAXS, and Impedance Spectroscopy

ESRF BM26 - Assessing HSIL zeolite crystallization in mixed cation systems

Cite this