Local structure and magnetism of Co3+ in wurtzite Co:ZnO

Bastian Henne, Verena Ney, Julia Lumetzberger, K. Ollefs, F. Wilhelm, A. Rogalev, Andreas Ney

Research output: Contribution to journalArticlepeer-review

Abstract

The structural and magnetic properties of 30% and 50% Co-doped ZnO have been investigated in order to determine the influence of the presence of Co3+ as a potential p-type dopant. For 30% doping, Co3+ could be stabilized in the wurtzite lattice of ZnO without phase separation by providing high oxygen partial pressures during growth. At 50% Co concentration, the crystal lattice destabilizes. X-ray absorption spectroscopy and simulations are used to substantiate the valence and local structure of Co3+. Integral and element selective magnetometry reveals uncompensated antiferromagnetism of the Co atoms irrespective of being present as Co2+ or Co3+.
Original languageEnglish
Article number054406
Pages (from-to)054406
Number of pages7
JournalPhysical Review B: Condensed Matter and Materials Physics
Volume95
Issue number5
DOIs
Publication statusPublished - 2017

Fields of science

  • 210006 Nanotechnology
  • 103 Physics, Astronomy
  • 103011 Semiconductor physics
  • 103018 Materials physics
  • 202032 Photovoltaics
  • 103009 Solid state physics
  • 103017 Magnetism

JKU Focus areas

  • Engineering and Natural Sciences (in general)

Cite this